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184 F. J. Duarte
a
b
Coaxial flashlamp dye laser
FIGURE 8
(Reprinted with permission from Duarte et a/. [72] and Elsevier Science.)
Schematics of (a) flashlamp-pumped MPL oscillator and (b) HMPGI oscillator.
In this regard, the narrow-linewidth emission pulse must be synchronized to
arrive during the buildup period of the forced-oscillator pulse. In the case of
forced oscillators using unstable resonator optics, the magnification of the optics
must be optimized relative to the beam dimensions of the master oscillator to
completely fill the active volume of the forced oscillator. Also. the injection beam
should be aligned exactly for concentric propagation along the optical axis of
the forced oscillator. The performance of flashlamp-pumped master-oscillator/
forced-oscillator systems is listed in Table 10. In addition to those results, energy
gains as high as 478 have been reported for an MPL master oscillator and a
forced oscillator with a magnification factor of 5 [62].
The use of cw dye laser oscillators as injection sources of amplification
stages utilizing ring cavity configurations is discussed by Blit et al. [78] and Trehin et a/. [79].
4. cw LASER-PUMPED DYE LASERS
The cw dye lasers span the spectrum from -370 to -1000 nm. Frequency
doubling extends their emission range into the 260- to 390-nm region. An important feature of cw dye lasers has been their ability to yield extremely stable
emissions and very narrow linewidths. These qualities have made cw dye lasers
5 Dye Lasers 185
FIGURE 9
sion from Duarte et al. [72] and Elsevier Science.)
Partial view of ruggedized multiple-prism grating oscillator. (Reprinted with permisMaster
oscillator
Forced
oscillator
Grating
FIGURE 1 0 Master-oscillator/forced-oscillator system. (Reprinted with permission from
Duarte and Conrad 1731.)
extremely important to applications in physics, spectroscopy, and other sciences.
A thorough and extensive description of this branch of dye lasers is given by
Hollberg [3]. Here some of the most important features of cw dye lasers and
their emission characteristics are surveyed.
4.1 Excitation Sources for cw Dye Lasers
The main sources of excitation for cw dye lasers are the argon ion (AI-+) and
the krypton ion (Kr+) lasers. These are conventional discharge lasers that emit
186 F.J. Duarte
TABLE 8
Master Oscillatora
Optimum Performance of Ruggedized Multiple-Prism Grating
Output energy (mJ) A\’ (hIHz) 6%’h AB (mrad) C (rnkl)
2.2-3.6 300 4.63 x 10-7 0.35 0.01
aFrom Duarte er al. [72], with permission.
TABLE 9 Performance of Ruggedized Multiple-Prism Grating Master
Oscillator Prior (First Row) and Following (Second Row) Field Testa
Output energy (mJ) Av (MHz) 6k% AB (mrad) C (mhl)
2-3
2-3
300 1.45 x 10-6 0.51 0.01
300 1.18 x 10-6 0.45 0.01
.From Duarte et al. [72]. with permission
TABLE 1 0
Forced-Oscillator Systems0
Performance of Flashlamp-Pumped Master-Oscillator/
Forced-oscillator output
blaster oscillator configuration energy Energy gain Reference
Tso etalons Flat-mirror cavity 600 mJ at 589 nm 200 [751
Three etalons Planoconcave resonaior 3J -267 [761
Trio etalons Flat-mirror cavity 300 mJ at 590 nm [771
A\, = 8.65 GHz
i2v = 4 GH2
A\’ = 346 MHz
MPL Positive-branch unstable resonator 600 mJ at 590 nm 60 ~731
Av 5 175 MHz
OXdapted from Duarte [37]. with permission.
via excitation mechanisms such as Penning ionization [go]. Table 11 lists some
of the most widely used transitions in dye laser excitation. Note that the quoted
powers are representative of devices available commercially. It should also be
indicated that not all transitions may be available simultaneously and that more
than one set of mirrors may be required to achieve lasing in different regions of
the spectrum. Also, for a mirror set covering a given spectral region, lasing of
individual lines may be accomplished using intracavity prism tuners.
5 Dye Lasers 187
TABLE 1 1 Excitation Lasers of cw Dye Lasers
Laser Transitiona Wavelength (nm) Powerb (W)
5p4p;. - .5s2P,,,
5p4P9: - 5s4Px,i
5p4PQ1 - 5S4P,,>
.5p4Do, - 5S2P,,?
528.69
514.53
501.72
496.51
487.99
476.49
472.69
465.79
457.93
4.54.50
799.32
752.55
676.4
647.09
568.19
530.87
520.83
1.5
10.0
1 .s
2.5
7.0
2.8
1.2
0.75
1.4
1 .o
0.1
0.35
0.2
1.4
0.53
0.7
0.25
~~~~~~~~ ~~~~ ~ ~ ~
OTransition identification from [SO].
hAr+ laser power from [3] and Kr+ laser powers from [81]
Given the relatively long cavity length of these lasers (typically -1 m), and
their narrow beamwaists (-1 mm), the output beam characteristics are excellent.
In this regard these 1a.sers can offer single-transverse-mode outputs and beam
divergence’s approaching the diffraction limit.
In addition to the output powers listed in Table 11, higher powers are available. For instance, Baving et al. [82] reports the use of a 200-W multiwavelength A@ laser in the excitation of a linear cw dye laser. The Ar+ laser oscillated
simultaneously at 457.93, 476.49,487.99,496.51, 501.72, and 514.53 nm. Other
lasers useful in the excitation of cw dye lasers include HeNe [83,84], frequencydoubled cw Nd:YAG [3], and semiconductor lasers.
4.2 cw Dye Laser Cavities
The cw dye laser cavities evolved from the simple and compact linear cavity
first demonstrated by Peterson et al. [85]. External mirrors and intracavity tuning
prisms were introduced by Hercher and Pike [86] and Tuccio and Strome [25]
(Fig. 11). An important innovation in cw dye lasers was the introduction of the
dye jet [83]. Fast flow of the dye solution at speeds of a few m-s-1 is important
188 F. J. Duarte
Stainless
Brewster
Angle Prism
Argon Laser Beam
514.5 nm
Dye Laser
Beam
FIGURE 1 1
and Strome [XI.)
Linear cw dye laser cavity configuration. (Reprinted 41th permission from Tuccio
to induce heat dissipation and hence reduce thermally induced optical inhomogeneities in the active medium [85].
Widely used configurations of cur dye laser cavities include the three-mirror
folded linear cavity (see, for example, [20] and references therein) and ring-dye
laser cavities (see, for example, [3] and references therein). These two configurations are shown in Fig. 12. In both cases excitation from a cw laser is accomplished semilongitudinally to the optical axis defined by M, and M,. Tuning elements. or frequency-selective elements (FSEs), are deployed between h/I, and
M, in the linear cavity, and between M, and M, in the ring cavity. The unidirectional device (UDD) depicted in Fig. 12(b) is an optical diode that controls the
direction of propagation in the ring cavity [3].
Ring-dye laser cavities circumvent the problem of spatial hole burning associated with linear cavities [3]. Also ring cavities are reported to yield higher singlelongitudinal-mode power than linear cavities [3]. However, linear configurations
offer greater optical simplicity and lower oscillation thresholds.
Diels [87] discusses the use of propagation matrices, applicable for Gaussian beam propagation analysis, to characterize stability conditions and astigmatism in cw dye laser cavities.
Linewidth narrowing and FSEs used in cw dye lasers are birefringent crystals. prisms, gratings, and Fabry-Perot etalons. Often two or more FSEs are necessary to achieve single-longitudinal-mode oscillation. The first stage in the frequency narrowing usually consists of utilizing prisms or birefringement filters to
yield a bandwidth compatible with the free spectral range (FSR) of the first of
two etalons. In turn, the second etalon has a FSR and finesse necessary to restrict
oscillation in the cavity to a single-longitudinal mode [3]. Alternative approaches
may replace the second etalon by an interferometer [88]. The performance of various linear and ring cw dye lasers is listed in Table 12.